$In\ situ$ gas monitoring by fiber-coupled Raman spectrometry for H$_2$-risk management in nuclear containment during a severe nuclear aAccident - CEA - Commissariat à l’énergie atomique et aux énergies alternatives Accéder directement au contenu
Article Dans Une Revue IEEE Transactions on Nuclear Science Année : 2020

$In\ situ$ gas monitoring by fiber-coupled Raman spectrometry for H$_2$-risk management in nuclear containment during a severe nuclear aAccident

Résumé

During a severe nuclear accident leading up to core melting, molten corium-concrete interaction (MCCI) and core-coolant water reaction both release large amounts of hydrogen (H$_2$ ) gas in the containment atmosphere. According to the Shapiro-Moffette ternary diagram and depending on local partial pressures of H$_2$ , air, and water vapor, deflagration/detonation may occur with potential deleterious impact over equipment and structures. CO and CO$_2$ are also of interest, as revealing gases for MCCI. Pressurized Water Reactors (PWRs) of French Nuclear Power Plants (NPPs) are equipped with passive autocatalytic recombiners (PARs), partly mitigating the H$_2$ risk. However, the H$_2$ -risk management strategy may be significantly improved by performing in situ monitoring of H$_2$ , O$_2$ , N$_2$ , H$_2$O, CO, and CO$_2$ partial pressures at several locations inside the containment, to account for potential local combustion risk. Raman spectrometry (RS) involves only one laser and spectrometer equipped with a 2-D charge-coupled device (CDD). Raman probes are chemically selective and may be radiation-hardened. Custom-made fiber-coupled Raman probes, linked with a readout unit, were qualified in a climatic chamber, a flame-propagation tube, a $^{60}$Co irradiation cell, a 3-D shaking table, a steam jet and the MISTRA facility (1/10 reduced-scale containment mock-up dedicated to thermo-hydraulic tests).
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Dates et versions

cea-04385873 , version 1 (11-01-2024)

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Citer

Sylvain Magne, Simon Nehr, Xavier Buet, Ahmed Bentaïb, Emmanuel Porcheron, et al.. $In\ situ$ gas monitoring by fiber-coupled Raman spectrometry for H$_2$-risk management in nuclear containment during a severe nuclear aAccident. IEEE Transactions on Nuclear Science, 2020, 67 (4), pp.617-624. ⟨10.1109/TNS.2020.2965622⟩. ⟨cea-04385873⟩
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