Journal Articles Journal of Nuclear Materials Year : 2024

Impact of gold ions irradiation on the initial alteration rate of the International Simple Glass

Abstract

This study addresses the impact of 7 MeV Au irradiation on the initial alteration rate of International Simple Glass (ISG), considered as a reference for nuclear glasses. This irradiation scenario simulates the effect of nuclear collisions of the recoil nuclei of α decays. In order to study the very first moments of glass alteration, non-irradiated and Au ions irradiated ISG glass monoliths were altered in pure water at 90°C, pH 9 and with a ratio of glass surface area to solution volume of 0.01 cm$^{-1}$. Glass alteration was monitored by measuring the releases of the glass elements in solution by UV-visible spectrophotometry and Inductively Coupled Plasma-Atomic Emission Spectroscopy (ICP-AES). Under these alteration conditions, the releases of the elements in solution are congruent. The initial alteration rate was found to be (2.0 ± 0.8) times higher for the irradiated glass monoliths than for non-irradiated samples.
Fichier principal
Vignette du fichier
article_JNM_C. Gillet.pdf (1.24 Mo) Télécharger le fichier
Origin Files produced by the author(s)

Dates and versions

cea-04844467 , version 1 (17-12-2024)

Identifiers

Cite

Célia Gillet, Stephanie Szenknect, Magaly Tribet, Hélène Arena, Sylvain Peuget. Impact of gold ions irradiation on the initial alteration rate of the International Simple Glass. Journal of Nuclear Materials, 2024, 588, pp.154817. ⟨10.1016/j.jnucmat.2023.154817⟩. ⟨cea-04844467⟩
24 View
4 Download

Altmetric

Share

More